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Split Complementery is choosing one color on the color wheel and using each color on each side of its complement (the color directly across the color you chose).
Left: In this chart I chose Cobalt Blue and its complements are Cad. Yellow Deep and Permamnet Red which are the two colors on each side of Warm Orange--the exact complement of Cobalt Blue.
Right: Pthalo Green and its split complements Permanent Red, and Magenta (New Orleans Red-Violet)
I'm using Terry Madden Paints and the Terry Madden Color Clock as my guide.