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PLA-PHB blends

Snapshot from an atomistic molecular dynamics (MD) simulation of polylactide (PLA) and polyhydroxybutyrate (PHB) blend. The full simulation time was over a microsecond.

 

The simulations show that PLA and PHB are miscible. More interestingly, however, the simulations show the existence of two glass transitions in the blends: 1) at the scale of a few Kuhn lengths and 2) second transition at a longer time scale. Thus, the miscibility of the blends depends on the length scale.

 

Reference:

 

Scale-Dependent Miscibility of Polylactide and polyhydroxybutyrate: Molecular Dynamics Simulations, A. Glova, S. Falkovich, S. Dmitrienko, A. Lyulin, S. Larin, V. Nazaraychev, Mikko Karttunen, S. Lyulin, Macromolecules, 51, 552-563 (2018).

 

WWW: dx.doi.org/10.1021/acs.macromol.7b01640

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Uploaded on March 29, 2018